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• W2802238571 startingPage "13241" @default.
• W2802238571 abstract "Organic-inorganic hybrid perovskites are developed to pursue high charge carrier mobility and light absorption coefficient. In this study, we present a detailed comparative research of the atomic and electronic structures of single-layered perovskites (C4H9NH3)2PbBr4 with two-dimensional/three-dimensional (2D/3D) spatial arrangement to predict the in plane charge carrier mobility along with the charge effective mass, elastic constant, and deformation potential. The calculated results reveal that the intrinsic in plane carrier mobilities of 2D single-layered hybrid perovskite (C4H9NH3)2PbBr4 along the 100 and 010 directions are superior to those of the 3D structure. Furthermore, the optical properties are calculated from the electronic structure; it is found that the light absorption spectrum of 2D single-layered perovskite (C4H9NH3)2PbBr4 with a high absorption coefficient is wider than that of the 3D phase. We speculate that the superior mobility and wider absorption spectrum of the 2D mono-layered perovskite are due to high charge density and ferroelectricity originating from structure distortion upon 3D-to-2D structure transformation. These results indicate that the 2D single-layered hybrid perovskite (C4H9NH3)2PbBr4 is a potential candidate for application in the optoelectronic and photovoltaic fields." @default.
• W2802238571 created "2018-05-17" @default.
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• W2802238571 date "2018-01-01" @default.
• W2802238571 modified "2023-10-15" @default.
• W2802238571 title "High transport and excellent optical property of a two-dimensional single-layered hybrid perovskite (C₄H₉NH₃)₂PbBr₄: a theoretical study" @default.
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• W2802238571 doi "https://doi.org/10.1039/c8cp01573b" @default.
• W2802238571 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29726869" @default.
• W2802238571 hasPublicationYear "2018" @default.
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