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• W2802383179 abstract "We have demonstrated the solid-state formation of a uranyl peroxide (UP) species from hydrated uranyl fluoride via a uranyl hydroxide intermediate, the first observation of a UP species formed in a solid-state reaction. Water vapor pressure is shown to be a driving factor of both the loss of fluorine and the subsequent formation of peroxo units. We have ruled out a photochemical mechanism for formation of the UP species by demonstrating that the same reaction occurs in the dark. A radiolytic mechanism is unlikely because of the low radioactivity of the sample material, suggesting the existence of a novel UP formation mechanism." @default.
• W2802383179 created "2018-05-17" @default.
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• W2802383179 date "2018-05-10" @default.
• W2802383179 modified "2023-09-25" @default.
• W2802383179 title "Evidence of a Nonphotochemical Mechanism for the Solid-State Formation of Uranyl Peroxide" @default.
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• W2802383179 doi "https://doi.org/10.1021/acs.inorgchem.8b00512" @default.
• W2802383179 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29745654" @default.
• W2802383179 hasPublicationYear "2018" @default.
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