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• W2802486314 abstract "Abstract An aromatic lactam acceptor unit, thieno[3,2‐c]isoquinolin‐5(4H)‐one (TIQ), is developed. Compared with its analogues, dithieno[3,2‐b:2′,3′‐d]pyridin‐5(4H)‐one (DTP) and phenanthridin‐6(5H)‐one (PN), TIQ shows its advantage in constructing donor–acceptor (D–A) copolymers for efficient solar cells. TIQ‐based D–A copolymer PTIQ4TFBT delivers a power conversion efficiency (PCE) of 10.16% in polymer:fullerene solar cells, while those based on DTP and PN copolymers, PDTP4TFBT and PPN4TFBT, afford PCEs around 8.5%. The higher performance of PTIQ4TFBT:PC 71 BM solar cells originates from enhanced short‐circuit current density ( J sc ) and fill factor (FF), because of favorable morphology, less bimolecular recombination, and balanced charge transport in the active layer. Moreover, the performance for PTIQ4TFBT:PC 71 BM solar cells is less sensitive to active layer thickness than PDTP4TFBT:PC 71 BM and PPN4TFBT:PC 71 BM solar cells. Over 8% PCEs can be obtained from PTIQ4TFBT:PC 71 BM solar cells when the active layer thickness is over 500 nm." @default.
• W2802486314 created "2018-05-17" @default.
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• W2802486314 date "2018-04-19" @default.
• W2802486314 modified "2023-10-14" @default.
• W2802486314 title "A Thieno[3,2-c]Isoquinolin-5(4H)-One Building Block for Efficient Thick-Film Solar Cells" @default.
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• W2802486314 doi "https://doi.org/10.1002/aenm.201800397" @default.
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