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• W2802556263 startingPage "10156" @default.
• W2802556263 abstract "Abstract Multifunctional cyclopentadiene (Cp) ligands and their rhenium and 99m Tc complexes were prepared by a versatile synthetic route. The properties of these Cp ligands can be tuned on demand, either during their synthesis (variation of R 1 ) or through post‐synthetic functionalization with two equal or different vectors (V 1 and V 2 ). Variation of these groups enables a combinatorial approach in the synthesis of bioorganometallic complexes. This is demonstrated by the preparation of Cp ligands containing both electron‐donating and electron‐withdrawing groups at the R 1 position and their subsequent homo‐ or heterofunctionalization with biovector models (benzylamine and phenylalanine) under standard amide bond‐formation conditions. All ligands can be coordinated to the fac ‐[Re(CO) 3 ] + and fac ‐[ 99m Tc(CO) 3 ] + cores to give tetrafunctional complexes in straightforward and functional‐group‐tolerant procedures. The 99m Tc complexes were prepared in one step, in 30 min, and under aqueous conditions from generator‐eluted [ 99m TcO 4 ] − ." @default.
• W2802556263 created "2018-05-17" @default.
• W2802556263 creator A5002135335 @default.
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• W2802556263 date "2018-06-21" @default.
• W2802556263 modified "2023-10-17" @default.
• W2802556263 title "Multifunctional Cyclopentadienes as a Scaffold for Combinatorial Bioorganometallics in [(η⁵‐C₅H₂R₁R₂R₃)M(CO)₃] (M=Re, ^99mTc) Piano‐Stool Complexes" @default.
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• W2802556263 doi "https://doi.org/10.1002/chem.201801271" @default.
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