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• W2802712609 abstract "Abstract A rational and effective strategy for the synthesis of a high‐performance non‐precious metal electrocatalyst for oxygen reduction reaction (ORR) was developed by inducing reconstruction of Fe‐N x site on pig‐bone‐derived nitrogen‐doped hierarchically porous carbon. The resultant Fe/N‐doped carbon electrocatalyst possessed abundant atomically dispersed non‐planar Fe‐N 4 ORR active sites, with absolute presence of active D1 (Fe II ‐N 4 ) and D3 (N‐Fe II ‐N 2+2 ) sites, as well as large specific surface area and three‐dimensional porous structure with hierarchical micro‐/meso‐/macro‐pore distribution, which increased the utilization of active sites and promoted mass transport of ORR reactants. This resulted in a remarkably superior ORR activity with half‐wave potential of 0.87 V (20 mV higher than Pt/C) and kinetic current density of 10.9 mA cm −2 at 0.85 V (2.3‐fold of Pt/C) in alkaline electrolyte. This methodology provides a route for atomic‐level design of high‐performance ORR electrocatalyst." @default.
• W2802712609 created "2018-05-17" @default.
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• W2802712609 date "2018-06-01" @default.
• W2802712609 modified "2023-09-30" @default.
• W2802712609 title "Towards High-Performance Electrocatalysts for Oxygen Reduction: Inducing Atomic-Level Reconstruction of Fe-N_<i>x</i> Site for Atomically Dispersed Fe/N-Doped Hierarchically Porous Carbon" @default.
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• W2802712609 doi "https://doi.org/10.1002/chem.201800937" @default.
• W2802712609 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29682804" @default.
• W2802712609 hasPublicationYear "2018" @default.
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