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- W2803067314 abstract "Porous single crystals are promising candidates for solar fuel production owing to their long range charge diffusion length, structural coherence, and sufficient reactive sites. Here, a simple template-free method of growing a selectively branched, 2D anatase TiO2 porous single crystalline nanostructure (PSN) on fluorine-doped tin oxide substrate is demonstrated. An innovative ion exchange–induced pore-forming process is designed to successfully create high porosity in the single-crystalline nanostructure with retention of excellent charge mobility and no detriment to crystal structure. PSN TiO2 film delivers a photocurrent of 1.02 mA cm−2 at a very low potential of 0.4 V versus reversible hydrogen electrode (RHE) for photo-electrochemical water splitting, closing to the theoretical value of TiO2 (1.12 mA cm−2). Moreover, the current–potential curve featuring a small potential window from 0.1 to 0.4 V versus RHE under one-sun illumination has a near-ideal shape predicted by the Gartner Model, revealing that the charge separation and surface reaction on the PSN TiO2 photoanode are very efficient. The photo-electrochemical water splitting performance of the films indicates that the ion exchange–assisted synthesis strategy is effective in creating large surface area and single-crystalline porous photoelectrodes for efficient solar energy conversion." @default.
- W2803067314 created "2018-05-17" @default.
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- W2803067314 date "2018-04-16" @default.
- W2803067314 modified "2023-10-17" @default.
- W2803067314 title "2D Porous TiO <sub>2</sub> Single‐Crystalline Nanostructure Demonstrating High Photo‐Electrochemical Water Splitting Performance" @default.
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- W2803067314 doi "https://doi.org/10.1002/adma.201705666" @default.
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