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- W2803335343 abstract "Green and efficient procedures are essential for the chemoselective hydrogenation of functionalized nitroarenes to form industrially important anilines. Herein, it is shown that visible-light-driven, chemoselective hydrogenation of functionalized nitroarenes with groups sensitive to forming anilines can be achieved in good to excellent yields (82–100 %) in water under relatively mild conditions and catalyzed by low-cost and recyclable graphitic carbon nitride. The process is also applicable to gram-scale reaction, with a yield of aniline of 86 %. A study of the mechanism reveals that visible-light-induced electrons are responsible for the hydrogenation reactions, and thermal energy can also promote the photocatalytic activity. A study of the kinetics shows that this reaction possibly occurs through one-step hydrogenation or stepwise condensation routes. A wide range of applications can be expected for this green, efficient, and highly selective photocatalysis system in reduction reactions for the synthesis of fine chemicals." @default.
- W2803335343 created "2018-06-01" @default.
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- W2803335343 date "2018-07-04" @default.
- W2803335343 modified "2023-10-16" @default.
- W2803335343 title "Visible-Light-Driven Chemoselective Hydrogenation of Nitroarenes to Anilines in Water through Graphitic Carbon Nitride Metal-Free Photocatalysis" @default.
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- W2803335343 doi "https://doi.org/10.1002/asia.201800515" @default.
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