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- W2803554414 abstract "Chemistry studies the composition, structure, properties, and transformation of matter. A mechanistic understanding of the pertinent processes is required to translate fundamental knowledge into practical applications. The current development of ultrafast Raman as a powerful time-resolved vibrational technique, particularly femtosecond stimulated Raman spectroscopy (FSRS), has shed light on the structure–energy–function relationships of various photosensitive systems. This Perspective reviews recent work incorporating optical innovations, including the broad-band up-converted multicolor array (BUMA) into a tunable FSRS setup, and demonstrates its resolving power to watch metal speciation and photolysis, leading to high-quality thin films, and fluorescence modulation of chimeric protein biosensors for calcium ion imaging. We discuss advantages of performing FSRS in the mixed time–frequency domain and present strategies to delineate mechanisms by tracking low-frequency modes and systematically modifying chemical structures with specific functional groups. These unique insights at the chemical-bond level have started to enable the rational design and precise control of functional molecular machines in optical, materials, energy, and life sciences." @default.
- W2803554414 created "2018-06-01" @default.
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- W2803554414 creator A5082019030 @default.
- W2803554414 date "2018-05-25" @default.
- W2803554414 modified "2023-10-02" @default.
- W2803554414 title "Capturing Structural Snapshots during Photochemical Reactions with Ultrafast Raman Spectroscopy: From Materials Transformation to Biosensor Responses" @default.
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- W2803554414 doi "https://doi.org/10.1021/acs.jpclett.8b00373" @default.
- W2803554414 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29799757" @default.
- W2803554414 hasPublicationYear "2018" @default.
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