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- W2803892944 abstract "Abstract N‐Deprotonated five‐, six‐, seven, and nine‐membered lactams undergo smooth palladium‐catalyzed N‐allylation with methyl‐(pent‐3‐en‐2‐yl)‐carbonate or 2‐chloro‐3‐pentene. With axially chiral bisphosphane ligands, enantioselectivities ranging from 83 to 97% ee are reached. The configuration of one of the allylation products is assigned unambiguously by the preparation of a relay compound and by analogy to the others. Using the enantioselective allylation protocol as a key step, δ‐valerolactam is converted into (4 S ,9a R )‐4‐methylquinolizidine." @default.
- W2803892944 created "2018-06-01" @default.
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- W2803892944 date "2018-05-14" @default.
- W2803892944 modified "2023-10-12" @default.
- W2803892944 title "Enantioselective Palladium‐Catalyzed N‐Allylation of Lactams" @default.
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- W2803892944 doi "https://doi.org/10.1002/slct.201801233" @default.
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