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- W2804047340 abstract "This study reports the preparation of functional bioinorganic hybrid materials exhibiting catalytic activity and photoluminescent properties arising from the combination of enzymes and freestanding silicon-based nanoparticles. The hybrid materials reported herein have potential applications in biological sensing/imaging and theranostics, as they combine long-lived silicon-based nanoparticle photoluminescence with substrate-specific enzymatic activity. Thermal hydrosilylation of undecenoic acid and alkene-terminated poly(ethylene oxide) with hydride-terminated silicon nanocrystals afforded nanoparticles functionalized with a mixed surface made up of carboxylic acid and poly(ethylene oxide) moieties. These silicon-based nanoparticles were subsequently conjugated with prototypical enzymes through the carbodiimide-mediated amide coupling reaction in order to form bioinorganic hybrids that display solubility and photostability in phosphate buffer, photoluminescence (λmax = 630 nm), and enzymatic activity. They were characterized using Fourier transform infrared spectroscopy (FTIR), X-ray photoelectron spectroscopy (XPS), transmission electron microscopy (TEM), dynamic light scattering analysis (DLS), photoluminescence spectroscopy, and pertinent enzyme activity assays." @default.
- W2804047340 created "2018-06-01" @default.
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- W2804047340 date "2018-05-14" @default.
- W2804047340 modified "2023-09-24" @default.
- W2804047340 title "Functional Bioinorganic Hybrids from Enzymes and Luminescent Silicon-Based Nanoparticles" @default.
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- W2804047340 doi "https://doi.org/10.1021/acs.langmuir.8b01119" @default.
- W2804047340 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29758156" @default.
- W2804047340 hasPublicationYear "2018" @default.
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