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- W2804631023 abstract "This paper describes an unexplored property of conductive metal–organic frameworks (MOFs) as ion-to-electron transducers in the context of potentiometric detection. Several conductive two-dimensional MOF analogues were drop-cast onto a glassy carbon electrode and then covered with an ion-selective membrane to form a potentiometric sensor. The resulting devices exhibited excellent sensing properties toward anions and cations, characterized by a near-Nernstian response and over 4 orders of magnitude linear range. Impedance and chronopotentiometric measurements revealed the presence of large bulk capacitance (204 ± 2 μF) and good potential stability (drift of 11.1 ± 0.5 μA/h). Potentiometric water test and contact angle measurements showed that this class of materials exhibited hydrophobicity and inhibited the formation of water layer at the electrode/membrane interface, resulting in a highly stable sensing response with a potential drift as low as 11.1 μA/h. The property of ion-to-electron transduction of conductive MOFs may form the basis for the development of this class of materials as promising components within ion-selective electrodes." @default.
- W2804631023 created "2018-06-01" @default.
- W2804631023 creator A5050706702 @default.
- W2804631023 creator A5056241529 @default.
- W2804631023 date "2018-05-24" @default.
- W2804631023 modified "2023-10-16" @default.
- W2804631023 title "Conductive Metal–Organic Frameworks as Ion-to-Electron Transducers in Potentiometric Sensors" @default.
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- W2804631023 doi "https://doi.org/10.1021/acsami.8b03956" @default.
- W2804631023 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29792413" @default.
- W2804631023 hasPublicationYear "2018" @default.
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