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- W2805581723 abstract "Asymmetric amplification induced in the Soai autocatalytic reaction by chiral initiators that are enantiomeric only by virtue of an isotope, e.g., -CH3 vs CD3-, is examined by spectroscopic, kinetic, and DFT modeling studies to help understand requirements for the emergence of biological homochirality. We find that the initiator inhibits the autocatalytic pathway at the outset of the reaction but ultimately provides the imbalance required for asymmetric amplification. This work provides clues in the ongoing search for prebiotically plausible versions of asymmetric autocatalysis." @default.
- W2805581723 created "2018-06-13" @default.
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- W2805581723 date "2018-06-06" @default.
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- W2805581723 title "Rationalization of Asymmetric Amplification via Autocatalysis Triggered by Isotopically Chiral Molecules" @default.
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- W2805581723 doi "https://doi.org/10.1021/acscentsci.8b00297" @default.
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