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• W2805588771 endingPage "2937" @default.
• W2805588771 startingPage "2925" @default.
• W2805588771 abstract "Abstract A catalytic cascade has been developed for the synthesis of biaryl‐2‐methyl acetates via a palladium‐catalyzed ortho ‐C( sp 2 )−H bond arylation of pyruvate O ‐arylmethyl ketoximes with aryl iodides followed by a solvolysis, in which the pyruvic ketoxime ester as a new auxiliary is employed to direct the C( sp 2 )−H bond activation. The straightforward treatment of O ‐arylmethyl hydroxylamines and ethyl pyruvate with aryl iodides also provides the target products in a one‐pot fashion. Furthermore, the new palladacycle intermediate is unambiguously confirmed by single‐crystal X‐ray diffraction analysis. A plausible reaction pathway is proposed for the Pd‐catalyzed arylation‐acetolysis sequence. magnified image" @default.
• W2805588771 created "2018-06-13" @default.
• W2805588771 creator A5006265220 @default.
• W2805588771 creator A5046597133 @default.
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• W2805588771 creator A5048669408 @default.
• W2805588771 creator A5058394999 @default.
• W2805588771 creator A5071740901 @default.
• W2805588771 creator A5079166135 @default.
• W2805588771 creator A5082452057 @default.
• W2805588771 date "2018-06-25" @default.
• W2805588771 modified "2023-09-27" @default.
• W2805588771 title "Catalytic Cascade Access to Biaryl-2-Methyl Acetates from Pyruvate<i>O</i>-Arylmethyl Ketoximes<i>via</i>the Palladium-Catalyzed C(<i>sp</i>²)H Bond Arylation and C−O Bond Solvolysis" @default.
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