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• W2805820106 abstract "With the successful preparation of γ-alumina with high-energy external surfaces such as {111} facets, the crystal-facet effect of γ-Al2O3 on surface-loaded CrOx has been explored for semihydrogenation of acetylene. Our results indeed demonstrate that the harmonious interaction of CrOx with traditional γ-Al2O3, the external surfaces of which are typically low-energy{110} facets, has caused a highly efficient performance for semihydrogenation of acetylene over CrOx/(110)γ-Al2O3 catalyst, whereas the activity of the CrOx/(111)γ-Al2O3 catalyst for acetylene hydrogenation is suppressed dramatically due to the limited formation of active Cr species, restrained by the high-energy {111} facets of γ-Al2O3. Furthermore, the use of inexpensive CrOx as the active component for semihydrogenation of acetylene is an economically friendly alternative relative to commercial precious Pd catalysts. This work sheds light on a strategy for exploiting the crystal-facet effect of the supports to purposefully tailor the catalytic properties." @default.
• W2805820106 created "2018-06-13" @default.
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• W2805820106 date "2018-06-06" @default.
• W2805820106 modified "2023-10-18" @default.
• W2805820106 title "Crystal-Facet Effect of γ-Al₂O₃ on Supporting CrO_<i>x</i> for Catalytic Semihydrogenation of Acetylene" @default.
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• W2805820106 doi "https://doi.org/10.1021/acscatal.8b01619" @default.
• W2805820106 hasPublicationYear "2018" @default.
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