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- W2806391886 abstract "Periploside A is the prototypical congener of the pregnane glycosides occurring in the Chinese medicinal plant Periploca sepium, featuring a unique seven-membered formyl acetal bridged spiro-orthoester (FABO) sugar linkage and potent immunosuppressive activities. This account details our efforts on the stereoselective construction of the FABO motif that has led to a successful total synthesis of periploside A. 1 Introduction 2 Attempts at Construction of the FABO Motif 2.1 Intermolecular Condensation and Transacetalation 2.2 Intramolecular Hydrogen Atom Transfer (HAT) Reaction 3 Synthesis of the FABO Motif Bearing the Unnatural Anomeric Configuration 4 Synthesis of the FABO Motif Bearing the Natural Anomeric Configuration 4.1 Unsuccessful Attempts 4.2 Final Solution 5 Conclusion" @default.
- W2806391886 created "2018-06-13" @default.
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- W2806391886 date "2018-05-28" @default.
- W2806391886 modified "2023-09-25" @default.
- W2806391886 title "Tackling the Challenge of the Total Synthesis of Periploside A" @default.
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- W2806391886 doi "https://doi.org/10.1055/s-0037-1610152" @default.
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