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- W280658629 abstract "We report a study of the spatial structure of ($sqrt{3}$ifmmodetimeselsetexttimesfi{}$sqrt{3}$)R30ifmmode^circelsetextdegreefi{} and (1.5ifmmodetimeselsetexttimesfi{}1.5)R18ifmmode^circelsetextdegreefi{} CO adsorbed on Cu (111), using the angle-resolved photoemission extended fine structure (ARPEFS) technique. The ARPEFS data were taken along the surface normal-emission direction with a sample temperature of 80 K. The CO molecule adsorbs on an atop site for both adsorption phases. Full multiple-scattering spherical-wave (MSSW) calculations were used to extract the C-Cu bond length and the first Cu-Cu layer spacing for each adsorption phase. The C-Cu bond length is 1.91(1) AA{} in the ($sqrt{3}$ifmmodetimeselsetexttimesfi{}$sqrt{3}$)R30ifmmode^circelsetextdegreefi{} phase and 1.91(2) AA{} in the (1.5ifmmodetimeselsetexttimesfi{}1.5)R18ifmmode^circelsetextdegreefi{} phase. The first layer Cu-Cu spacing is 2.07(3) AA{} in the ($sqrt{3}$ifmmodetimeselsetexttimesfi{}$sqrt{3}$)R30ifmmode^circelsetextdegreefi{} phase. The first layer Cu-Cu spacing in the (1.5ifmmodetimeselsetexttimesfi{}1.5)R18ifmmode^circelsetextdegreefi{} phase is 2.01(4) AA{}, a contraction of 3% from the clean metal value of 2.07 AA{}. We calculate the bending mode force constant (1.5ifmmodetimeselsetexttimesfi{}1.5)R18ifmmode^circelsetextdegreefi{} phase to be ${mathit{k}}_{mathrm{ensuremath{delta}}}$=2.2(1)ifmmodetimeselsetexttimesfi{}${10}^{mathrm{ensuremath{-}}12}$ dyn/cm rad from the above bond lengths combined with previously published infrared absorption frequencies. textcopyright{} 1996 The American Physical Society." @default.
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- W280658629 date "1996-10-15" @default.
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- W280658629 title "Spatial structure determination of (√3×√3)<i>R</i>30° and (1.5×1.5)<i>R</i>18° CO or Cu(111) using angle-resolved photoemission extended fine structure" @default.
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- W280658629 doi "https://doi.org/10.1103/physrevb.54.10862" @default.
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