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• W2806790930 startingPage "3618" @default.
• W2806790930 abstract "A practical catalytic method to synthesize β,β- and γ,γ-substituted amines by opening aziridines and azetidines, respectively, using alkenyl, alkynyl, or aryl/heteroaryl trifluoroborate salts is described. This reaction features simple open-flask reaction conditions, the use of transition-metal-free catalysis, complete regioselectivity, and high diastereoselectivity. Preliminary mechanistic studies suggest that carbocation formation is disfavored. Stereoretentive addition is favored with Brønsted acid present, while stereoinversion is favored in its absence, indicating divergent mechanisms." @default.
• W2806790930 created "2018-06-13" @default.
• W2806790930 creator A5010681723 @default.
• W2806790930 creator A5089005483 @default.
• W2806790930 date "2018-06-06" @default.
• W2806790930 modified "2023-10-18" @default.
• W2806790930 title "Branched Amine Synthesis via Aziridine or Azetidine Opening with Organotrifluoroborates by Cooperative Brønsted/Lewis Acid Catalysis: An Acid-Dependent Divergent Mechanism" @default.
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• W2806790930 doi "https://doi.org/10.1021/acs.orglett.8b01394" @default.
• W2806790930 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29874082" @default.
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