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- W2807010657 abstract "Nacre mimetics show great potential as mechanically robust, lightweight, and promising functional materials. Herein, we report a nanostructured nacre-mimetic hybrid framework, prepared via in situ self-polymerization of tannic acid (TA) and pyrrole monomer on cellulose nanofiber (CNF)-anchored graphene nanosheets (GNs), as a two-dimensional interconnected network (designated as [email protected]) to fabricate mechanically robust and thermally and electrically conductive composites. A unique network structure with a combination of conductive polypyrrole (PPy) protrusions and multiscale nanofibers/nanoplates was obtained, where the nanohybrid protrusions acted as bridges that link the adjacent GNs and nanofibers. As a result, a composite with low filler loading (10.0 wt%) exhibited advantages for the combination of all properties, i.e., enhanced electrical and thermal conductivity (6.52 S cm−1 and 7.81 W m−1 K−1), high tensile strength (217.9 MPa), and good toughness (19.6 MJ m−3). We attribute the enhancement of these properties to the construction of an interconnected [email protected] skeleton and the oriented “brick-and-mortar” structure based on GNs blocks and the polyvinyl alcohol matrix, in which a mechanically robust conductive network was constructed. We envision that the relevant functionalities can be integrated into stiff and strong bioinspired materials as flexible microelectronic candidates." @default.
- W2807010657 created "2018-06-13" @default.
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- W2807010657 date "2018-10-01" @default.
- W2807010657 modified "2023-09-24" @default.
- W2807010657 title "Mechanically robust nacre-mimetic framework constructed polypyrrole-doped graphene/nanofiber nanocomposites with improved thermal electrical properties" @default.
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- W2807010657 doi "https://doi.org/10.1016/j.matdes.2018.06.004" @default.
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