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- W2807316628 abstract "The development of cost-effective non-precious metal catalysts has attracted much research attention because of their high oxygen reduction reaction (ORR) performance. Herein, based on three kinds of carbon nanotubes (CNTs) with different oxygen content, we prepare three CNTs-based iron phthalocyanine (FePc) composites via only a simple physical method. In surprise, the FePc-CNTs composites with the most oxygen content exhibit the highest ORR catalytic activity in comparison with commercial Pt/C in alkaline media, especially its half-wave potential (E1/2) and durability as well as methanol tolerance. A large amount of experimental measurements show that these superb catalytic activities can be mainly attributed to the possible formation of novel interactions between FePc and oxidized CNTs. It not only provides more active sites, but also is in favor of stabilizing active centers and removing intermediates in catalytic process. This work displays the effects of oxygen content and roughness of CNTs on the interactions between FePc and CNTs and their important role in ORR catalysis, providing a new insight into simple application of carbons materials." @default.
- W2807316628 created "2018-06-13" @default.
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- W2807316628 date "2018-08-01" @default.
- W2807316628 modified "2023-10-11" @default.
- W2807316628 title "The effect of oxygen content of carbon nanotubes on the catalytic activity of carbon-based iron phthalocyanine for oxygen reduction reaction" @default.
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- W2807316628 doi "https://doi.org/10.1016/j.electacta.2018.05.183" @default.
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