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- W2808079767 abstract "Four derivatives of dithieno[2,3-d;2′,3′-d′]benzo[1,2-b;3,4-b′]dithiophene (DTmBDT) have been synthesized to investigate the correlation between molecular structure, thin-film organization, and charge-carrier transport. Phenyl or thiophene end-capped derivatives at alpha positions of the outer thiophenes of DTmBDT present vastly different optoelectronic properties in comparison with bay-position alkyl-chain-substituted DTmBDT, which was additionally confirmed by density functional theory simulations. The film morphology of the derivatives strongly depends on alkyl substituents, aromatic end-caps, and substrate temperature. Field-effect transistors based on DTmBDT derivatives with bay-substituted alkyl chains show the best performance within this studied series with a hole mobility up to 0.75 cm2/V s. Attachment of aromatic end-caps disturbs the ordering, limiting the charge-carrier transport. Higher substrate temperature during deposition of the DTmBDT derivatives with aromatic end-caps results in larger domains and improved the transistor mobilities but not beyond the alkylated DTmBDT." @default.
- W2808079767 created "2018-06-21" @default.
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- W2808079767 date "2018-06-18" @default.
- W2808079767 modified "2023-09-28" @default.
- W2808079767 title "Molecular Ordering of Dithieno[2,3-<i>d</i>;2′,3′-<i>d</i>]benzo[2,1-<i>b</i>:3,4-<i>b</i>′]dithiophenes for Field-Effect Transistors" @default.
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- W2808079767 doi "https://doi.org/10.1021/acsomega.8b00836" @default.
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