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- W2808187487 abstract "We report in this paper the N-heterocyclic carbene/transition metal and N-heterocyclic carbene/base cascade catalysis in the reaction of o-alkynylbenzaldehydes with N-acylimines, demonstrating the example of reaction pathways steered by catalysts. Under the catalysis of a thiazole carbene/Et3N followed by Cu(OAc)2 in acetonitrile at ambient temperature, o-alkynylbenzaldehydes underwent reaction with N-acylimines that were generated in situ from N-((aryl)(tosyl)methyl)amides to produce a pair of Z- and E-2-amido-3-benzylidene-1-indanones in 47–92% total yields. The reaction of the same substrates in the presence of a thiazole carbene and Cs2CO3, on the other hand, afforded (1E,3Z)-1-amidobenzylidene-3-benzylidene-1,3-dihydroisobenzofurans in 54–89% yields." @default.
- W2808187487 created "2018-06-21" @default.
- W2808187487 creator A5004314121 @default.
- W2808187487 creator A5051697029 @default.
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- W2808187487 date "2018-06-12" @default.
- W2808187487 modified "2023-09-26" @default.
- W2808187487 title "Selective Synthesis of Multifunctionalized 2,3-Dihydroinden-1-ones and 1,3-Dihydroisobenzofurans from the Reaction of <i>o</i>-Alkynylbenzaldehydes with Imines Steered by N-Heterocyclic Carbene/Copper(II) and N-Heterocyclic Carbene/Base Cascade Catalysis" @default.
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- W2808187487 doi "https://doi.org/10.1021/acs.joc.8b01163" @default.
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