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- W2808376384 abstract "Abstract An experimental and parametric behavior study of disproportionation and transalkylation between C8 aromatics and toluene were carried out over mono-functional acid Beta zeolite with a SiO2/Al2O3 ratio of 35 (BEA35). The experiments were performed in liquid phase under the following conditions: 453, 473, and 493 K and 2.1 MPa. Ethylbenzene disproportionation and ethylbenzene-toluene transalkylation were identified as the main side reactions; therefore, the kinetics of both reactions were estimated. Both reactions were verified to be second-order with no signs of competition for the adsorption sites under the studied conditions. Additionally, ethylbenzene disproportionation and ethylbenzene-toluene transalkylation, undergo through a deethylation-ethylation mechanism, the activation energies were 66 and 57 kJ/mol respectively. Furthermore, the existence of parallel reactions, as well as the feed concentration, showed no effect on the p-diethylbenzene selectivity. Selectivity towards the para-isomer was observed only at very low conversions. Finally, an analytical solution was developed for the system showing excellent agreement with the experimental data." @default.
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- W2808376384 date "2018-07-01" @default.
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- W2808376384 title "Xylene isomerization side reactions over Beta zeolite: Disproportionation and transalkylation of C8 aromatics and toluene" @default.
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- W2808376384 doi "https://doi.org/10.1016/j.apcata.2018.06.011" @default.
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