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• W2809663487 abstract "Metal-organic frameworks (MOFs) have gained tremendous attention in the fields of environmental restoration and sustainable energy for their potential use as photocatalyst. Herein, a new two-dimensional (2D) Cu(I)-based MOF material showing a narrow forbidden-band of 2.13 eV was successfully constructed using a visible-light-harvesting anthracene-based bipyridine ligand. The as-prepared MOF demonstrates high chemical stability and could be stable in the pH range 2-13, which is favorable for its potential application in photocatalysis. Photocatalytic experiments demonstrate that this Cu(I)-MOF exhibits high reactivity for reduction of Cr(VI) in water, with 95% Cr(VI) converting to Cr(III) in 10 min by using MeOH as scavenger under visible-light illumination. Furthermore, this MOF could behave as a highly active photocatalyst for H2 evolution without additional photosensitizers and cocatalyst. Remarkably, the as-prepared MOF shows enhanced photocatalytic Cr(VI) reduction and H2 evolution performances compared with the pristine light-harvesting ligand under the same conditions. In connection to these, the photocatalytic reaction mechanism has also been probed." @default.
• W2809663487 created "2018-06-29" @default.
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• W2809663487 date "2018-06-18" @default.
• W2809663487 modified "2023-10-17" @default.
• W2809663487 title "Stable Layered Semiconductive Cu(I)–Organic Framework for Efficient Visible-Light-Driven Cr(VI) Reduction and H₂ Evolution" @default.
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• W2809663487 doi "https://doi.org/10.1021/acs.inorgchem.8b01137" @default.
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• W2809663487 hasPublicationYear "2018" @default.
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