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- W2809964518 abstract "Three phosphine oxide functionalized pillar[5]arenes were dissolved in 1‐butyl‐3‐methylimidazolium bis(trifluoromethanesulfonyl)imide ([C 4 mim][Tf 2 N]), a room‐temperature ionic liquid, and the solutions were used to extract representative tri‐, tetra‐ and hexavalent actinide ions, namely Am 3+ , Pu 4+ and UO 2 2+ ions, from nitric acid feeds. Although the extraction of Am 3+ and UO 2 2+ ions decreased with increasing feed acid concentration, the opposite trend was observed for Pu 4+ . The extraction of the actinide ions followed the trend Pu 4+ > UO 2 2+ > Am 3+ at 3 m HNO 3 , and the extraction efficiency of the ligands followed the trend L III > L II > L I with decreasing spacer lengths. The extraction mechanism conformed to the “solvation” type usually encountered in the case of molecular diluents. The nature of the extracted species was ascertained by “slope analysis”, in which the ligand, nitrate ion and C 4 mim + ion concentrations were varied, as well as luminescence spectroscopic measurements. The possibility of recycling of the ionic‐liquid‐based solvent systems was evaluated by carrying out back‐extraction as well as radiolytic degradation studies." @default.
- W2809964518 created "2018-07-10" @default.
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- W2809964518 date "2018-08-28" @default.
- W2809964518 modified "2023-10-13" @default.
- W2809964518 title "Complexation of Actinides with Phosphine Oxide Functionalized Pillar[5]arenes: Extraction and Spectroscopic Studies" @default.
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- W2809964518 doi "https://doi.org/10.1002/ejic.201800576" @default.
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