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- W2810132243 abstract "Abstract Tourmaline, an economical and eco-friendly natural mineral, has been widely used during the water treatment processes. In this investigation, the raw tourmaline has been found to be effective as a catalyst for ozonation in the degradation of atrazine (ATZ) under low temperature (278 K). Within typical experimental conditions (tourmaline dosage = 1 g L−1, [ATZ]0 = 5 μM, [O3]0 = 3 mg L−1, at pH 7.0 and 278 K), the removal efficiency of ATZ in catalytic ozonation was 98% after 10 min, compared with only 27% ATZ removal in the absence of catalyst. Surface properties and components of tourmaline were characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), Fourier transform infrared spectra (FTIR), pyridine-FTIR and energy dispersive X-ray (EDX). The characterization studies showed that metal attached hydroxyl groups (M OH, M = Fe, Al and Si) were the main active sites for ozone adsorption and decomposition. The formation of hydroxyl radicals ( OH) as well as hydrogen peroxide (H2O2) led to fast ATZ degradation and 31 kinds of intermediates; meanwhile, possible degradation pathways of ATZ were detected and proposed. The mechanisms of reaction were proposed for tourmaline-catalyzed ozonation based on all the experimental results and material characterizations." @default.
- W2810132243 created "2018-07-10" @default.
- W2810132243 creator A5018434228 @default.
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- W2810132243 date "2018-12-01" @default.
- W2810132243 modified "2023-10-12" @default.
- W2810132243 title "Strong promoted catalytic ozonation of atrazine at low temperature using tourmaline as catalyst: Influencing factors, reaction mechanisms and pathways" @default.
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- W2810132243 doi "https://doi.org/10.1016/j.cej.2018.07.032" @default.
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