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- W2810358364 abstract "Exploring the crystallization process of metal oxide mesocrystals has attracted enormous attention recently. However, due to the lack of insight into the behaviors of short-lived species at initial growth stages, there is currently a gap in understanding the underlying growth mechanism. Here, a combination of a preseeded hydrothermal method and transmission electron microscopy allows us to witness the rapid crystallization by particle attachement (CPA) in the early growth stage of capsule-shaped rutile titania mesocrystals. The presence of the embryonic form of nanocapsules, the slight misalignment of the primary particles, and, most importantly, the atomic interface between primary particles during attachment strongly indicate the existence of CPA mechanism. Furthermore, we rationalize our findings in terms of the free energy landscapes that govern nonclassical formation pathways. Our study provides a practical approach to explore the formation mechanism of fast-growing crystals at their initial growth stages." @default.
- W2810358364 created "2018-07-10" @default.
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- W2810358364 date "2018-07-03" @default.
- W2810358364 modified "2023-10-16" @default.
- W2810358364 title "Early Stage Growth of Rutile Titania Mesocrystals" @default.
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- W2810358364 doi "https://doi.org/10.1021/acs.cgd.8b00028" @default.
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