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• W2810810144 abstract "Amphiphilic block copolymers consisting of hydrophobic regioregular head-to-tail (HT) chiral ((S)-poly-1a-b-poly-3) or achiral (poly-1b-b-poly-3) polythiophene chains and a hydrophilic poly(acrylic acid) chain were synthesized. (S)-Poly-1a-b-poly-3 with a chiral polythiophene block formed a micelle in water that exhibited a characteristic induced circular dichroism (ICD) in the π–π* transition region due to the formation of supramolecular π-stacked chiral aggregates of the chiral polythiophene blocks in the core. These aggregates were stable, showing no precipitation for more than 5 days. Micelles consisting of chiral (S)-poly-1a-b-poly-3 and achiral poly-1b-b-poly-3 showed negative nonlinear effects on supramolecular chiral aggregate formation in the core. Chiral polythiophene aggregates formed in (S)-poly-1a-b-poly-3 micelle cores were stabilized by the crosslinking of poly(acrylic acid) blocks with diamines in the shell. The ICD intensity of the (S)-poly-1a-b-poly-3 micelle after shell crosslinking showed almost no change with temperature, while that before shell crosslinking decreased with increasing temperature." @default.
• W2810810144 created "2018-07-10" @default.
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• W2810810144 date "2018-06-30" @default.
• W2810810144 modified "2023-09-25" @default.
• W2810810144 title "Synthesis of Amphiphilic Block Copolymers Containing Chiral Polythiophene Chains and Their Micelle Formation and Chiroptical Properties" @default.
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• W2810810144 doi "https://doi.org/10.3390/polym10070718" @default.
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