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• W2810992488 abstract "We report the long-range orientational organization of water using polarization-resolved second harmonic scattering operated in a right-angle configuration. A transition is observed between the neat water orientational organization involving an azimuthal molecular orientation distribution towards a radial molecular orientation distribution when salt is added. These two orientational phases are quantitatively described using a molecular model of the second harmonic scattering response. It is observed that the long-range correlation present in the neat water phase abruptly disappears and is replaced by a shorter range correlation centered around the ions as the salt concentration is increased.Received 12 January 2018DOI:https://doi.org/10.1103/PhysRevLett.120.263001© 2018 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasCollective effects in clustersSecond order nonlinear optical processesAtomic, Molecular & Optical" @default.
• W2810992488 created "2018-07-10" @default.
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• W2810992488 date "2018-06-27" @default.
• W2810992488 modified "2023-10-18" @default.
• W2810992488 title "Salt-induced Long-to-Short Range Orientational Transition in Water" @default.
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• W2810992488 doi "https://doi.org/10.1103/physrevlett.120.263001" @default.
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