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- W2818334429 abstract "Efficient photoinduced electron transfer was observed across a [10]cycloparaphenylene ([10]CPP) moiety that serves as a rigid non-covalent bridge between a zinc porphyrin and a range of fullerenes. The preparation of iodo-[10]CPP is the key to the synthesis of a porphyrin-[10]CPP conjugate, which binds C60 , C70 , (C60 )2 , and other fullerenes (KA >105 m-1 ). Fluorescence and pump-probe spectroscopy revealed intramolecular energy transfer between CPP and porphyrin and also efficient charge separation between porphyrin and fullerenes, affording up to 0.5 μs lifetime charge-separated states. The advantage of this approach towards electron donor-acceptor dyads is evident in the case of dumbbell-shaped (C60 )2 , which gave intricate charge-transfer behavior in 1:1 and 2:1 complexes. These results suggest that [10]CPP and its cross-coupled derivatives could act as supramolecular mediators of charge transport in organic electronic devices." @default.
- W2818334429 created "2018-07-19" @default.
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- W2818334429 date "2018-09-03" @default.
- W2818334429 modified "2023-10-12" @default.
- W2818334429 title "A Supramolecular [10]CPP Junction Enables Efficient Electron Transfer in Modular Porphyrin–[10]CPP⊃Fullerene Complexes" @default.
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- W2818334429 doi "https://doi.org/10.1002/anie.201802443" @default.
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- W2818334429 hasPublicationYear "2018" @default.
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