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- W28337712 abstract "The quadrupole dissociation cross sections of molecular hydrogen from excited rovibronic levels (v{double_prime}, J{double_prime}) in the ground electronic state show narrow (predissociation) resonances associated with barrier states in the final (v{prime}, J{prime}) channels. Solutions of the time-dependent Schrodinger equation constructed with expanding-lattice methodology and finite-difference time propagation are employed in studying the dissociation dynamics through these states. Accurate numerical wave functions obtained in both position and momentum representations verify explicitly the formation of the classical Bethe front in the long-time limit, in accordance with causality, and indicate the absence of the time delay commonly associated with such resonances. Pictorial representations of the time-dependent wave function for applied field frequencies at and near resonance indicate the sense in which there is an apparent delay in the arrival of flux at the detector. Possible observation of the resonance-distorted Bethe front is discussed." @default.
- W28337712 created "2016-06-24" @default.
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- W28337712 date "1993-05-01" @default.
- W28337712 modified "2023-09-23" @default.
- W28337712 title "Pure quadrupole predissociation resonances in molecular hydrogen" @default.
- W28337712 hasPublicationYear "1993" @default.
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