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• W2835252382 abstract "Abstract The development of heterogeneous catalysts for the synthesis of pharmaceutically relevant compounds is always important for chemistry research. Here, we report a selective aerobic oxidation of aromatic and aliphatic amines to corresponding amides over a nanorod manganese oxide (NR‐MnO x ) catalyst. The kinetic studies reveal that the NR‐MnO x catalyzed amine‐to‐amide reaction proceeds the oxidative dehydrogenation of the amines into nitriles, followed by hydrolysis of nitrile into amides. The NR−MnO x exhibits fast kinetics and high selectivities in these steps, as well as hinders the by‐product formation. More importantly, the NR‐MnO x catalyst is stable and reusable in the continuous recycle tests with water as a sole by‐product, exhibiting superior sustainability and significant advancement to outperform the traditional amide production route in acidic or basic media with toxic by‐products." @default.
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• W2835252382 date "2018-07-26" @default.
• W2835252382 modified "2023-10-05" @default.
• W2835252382 title "Aerobic Activation of C‐H Bond in Amines Over a Nanorod Manganese Oxide Catalyst" @default.
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• W2835252382 doi "https://doi.org/10.1002/cctc.201801058" @default.
• W2835252382 hasPublicationYear "2018" @default.
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