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- W2861553399 abstract "By introducing [6,6]-phenyl-C61-butyric acid methyl ester as an effective additive in the perovskite precursor solution, we demonstrate a grain interface-engineering approach for universally increasing the efficiency of perovskite solar cells based on the printable triple mesoscopic structure of TiO2/ZrO2/carbon. These perovskite solar cells have advantages of low-cost and are easy to scale up, however the micrometer-thick mesoscopic layers and one-step dropping method challenge perovskite crystallization in such devices, resulting in non-ignorable charge-recombination loss. With adding an optimized 0.25 mg mL−1 PCBM into the perovskite precursor solution, we improve the champion PCE of PSCs using MAPbI3 perovskites from 8.58% to 12.36% and that of PSCs using MAPbI2.95(BF4)0.05 perovskites from 12.77% to 14.26%. We find that the PCBM additive affects the perovskite morphology, facilitates the photo-generated charge separation and suppresses the charge recombination in the device, thus yielding a universal improvement of MPSC performance. This work gives a new insight towards designing high performance perovskite solar cells." @default.
- W2861553399 created "2018-07-19" @default.
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- W2861553399 date "2018-11-01" @default.
- W2861553399 modified "2023-10-15" @default.
- W2861553399 title "Fullerene derivative as an additive for highly efficient printable mesoscopic perovskite solar cells" @default.
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- W2861553399 doi "https://doi.org/10.1016/j.orgel.2018.07.002" @default.
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