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- W2883011508 abstract "To obtain the photocatalyst composed by sulfur vacancies rich NiS and graphitic carbon nitride (g-C3N4), a simple method has been found for using coordination polymer as precursor. Based on this strategy, an effective composite photocatalyst, NiS@g-C3N4, is synthesized successfully through the calcination of a Ni2+ based coordination polymer with 2-mercapto-5-propylpyrimidine as ligand. In this photocatalyst, the NiS nanoparticles with small size disperse evenly in 2-mercapto-5-propylpyrimidine derived g-C3N4. Electron paramagnetic resonance (EPR) suggests there are a lot of sulfur vacancies in NiS@g-C3N4. NiS@g-C3N4 exhibits intensive adsorption in the near-infrared region, which endows NiS@g-C3N4 with promising photothermal effect. With a 980 nm laser as light source (0.44 W·cm–2), the aqueous dispersion of NiS@g-C3N4 exhibits a temperature elevation of 56.7 °C with photothermal conversion efficiency of 58.2%. Under irradiation of simulated solar light, without Pt co-catalyst, NiS@g-C3N4 possesses a pro..." @default.
- W2883011508 created "2018-08-03" @default.
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- W2883011508 date "2018-07-19" @default.
- W2883011508 modified "2023-10-02" @default.
- W2883011508 title "Coordination Polymer Derived NiS@g-C<sub>3</sub>N<sub>4</sub> Composite Photocatalyst for Sulfur Vacancy and Photothermal Effect Synergistic Enhanced H<sub>2</sub> Production" @default.
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- W2883011508 doi "https://doi.org/10.1021/acssuschemeng.8b02153" @default.
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