Matches in SemOpenAlex for { <https://semopenalex.org/work/W2883291241> ?p ?o ?g. }
- W2883291241 abstract "The possibility to exploit shaped ultrabroadband laser pulses for molecular coherent control offers a unique implementation of numerous nonlinear spectroscopic methods in one setup. Nonlinear processes, such as coherent Raman microscopy, second harmonic generation, or two-photon fluorescence, which have been applied in many different applications in both the material and life sciences, can be selectively addressed and optimized just by changing the phase imprinted by a programmable pulse shaper. Here, the experimental realization of this concept for multimodal nonlinear microscopy is discussed and the successful implementation of adaptive spectral focussing schemes not only for nonlinear Raman but also for difference frequency generation based mid-infrared (Mid-IR) spectroscopy using a single broadband pulse from a Ti:sapphire laser is shown. Flexible pulse shaping enables tuning of the resonance frequency and the spectral width of the excitation. By variation of the instantaneous frequency difference and the amount of chirp, the experiment can be optimized to achieve high resolution spectroscopy reaching up to 20 cm−1. Matching the resolution of the experiment with the linewidths of the sample on the other hand optimizes the contrast for imaging at high signal levels. The combination and flexible switching between Raman or mid-IR excitation for spectroscopy and microscopy is demonstrated on alkynes, polymer films, and skin tissue. The simple addition of this complementary modality to an existing nonlinear microscope is a further step toward an all-purpose laser excitation source for multimodal microscopy." @default.
- W2883291241 created "2018-08-03" @default.
- W2883291241 creator A5001640684 @default.
- W2883291241 creator A5021528092 @default.
- W2883291241 creator A5041317047 @default.
- W2883291241 date "2018-07-27" @default.
- W2883291241 modified "2023-10-18" @default.
- W2883291241 title "Invited Article: Coherent Raman and mid-IR microscopy using shaped pulses in a single-beam setup" @default.
- W2883291241 cites W1869204496 @default.
- W2883291241 cites W1963803441 @default.
- W2883291241 cites W1966760455 @default.
- W2883291241 cites W1969273505 @default.
- W2883291241 cites W1971752921 @default.
- W2883291241 cites W1973634282 @default.
- W2883291241 cites W1975393486 @default.
- W2883291241 cites W1976558482 @default.
- W2883291241 cites W1977762417 @default.
- W2883291241 cites W1977919076 @default.
- W2883291241 cites W1979221508 @default.
- W2883291241 cites W1979874110 @default.
- W2883291241 cites W1980814228 @default.
- W2883291241 cites W1994826110 @default.
- W2883291241 cites W2004487310 @default.
- W2883291241 cites W2016989399 @default.
- W2883291241 cites W2017252690 @default.
- W2883291241 cites W2023534334 @default.
- W2883291241 cites W2040960402 @default.
- W2883291241 cites W2046000266 @default.
- W2883291241 cites W2052206842 @default.
- W2883291241 cites W2055495373 @default.
- W2883291241 cites W2058687177 @default.
- W2883291241 cites W2060925749 @default.
- W2883291241 cites W2064471493 @default.
- W2883291241 cites W2064949909 @default.
- W2883291241 cites W2067969133 @default.
- W2883291241 cites W2071070545 @default.
- W2883291241 cites W2071918265 @default.
- W2883291241 cites W2075250515 @default.
- W2883291241 cites W2077013371 @default.
- W2883291241 cites W2088437254 @default.
- W2883291241 cites W2103341993 @default.
- W2883291241 cites W2104460891 @default.
- W2883291241 cites W2118795579 @default.
- W2883291241 cites W2119768555 @default.
- W2883291241 cites W2120119020 @default.
- W2883291241 cites W2120548956 @default.
- W2883291241 cites W2143386071 @default.
- W2883291241 cites W2144525188 @default.
- W2883291241 cites W2148691803 @default.
- W2883291241 cites W2160258306 @default.
- W2883291241 cites W2165405204 @default.
- W2883291241 cites W2175250902 @default.
- W2883291241 cites W2258990403 @default.
- W2883291241 cites W2429715568 @default.
- W2883291241 cites W2564836236 @default.
- W2883291241 cites W2605253479 @default.
- W2883291241 cites W2606101966 @default.
- W2883291241 cites W2753236824 @default.
- W2883291241 cites W2755556010 @default.
- W2883291241 cites W2800026792 @default.
- W2883291241 cites W2900690884 @default.
- W2883291241 cites W4213168521 @default.
- W2883291241 doi "https://doi.org/10.1063/1.5030062" @default.
- W2883291241 hasPublicationYear "2018" @default.
- W2883291241 type Work @default.
- W2883291241 sameAs 2883291241 @default.
- W2883291241 citedByCount "13" @default.
- W2883291241 countsByYear W28832912412018 @default.
- W2883291241 countsByYear W28832912412019 @default.
- W2883291241 countsByYear W28832912412020 @default.
- W2883291241 countsByYear W28832912412021 @default.
- W2883291241 countsByYear W28832912412022 @default.
- W2883291241 countsByYear W28832912412023 @default.
- W2883291241 crossrefType "journal-article" @default.
- W2883291241 hasAuthorship W2883291241A5001640684 @default.
- W2883291241 hasAuthorship W2883291241A5021528092 @default.
- W2883291241 hasAuthorship W2883291241A5041317047 @default.
- W2883291241 hasBestOaLocation W28832912411 @default.
- W2883291241 hasConcept C102755159 @default.
- W2883291241 hasConcept C110806042 @default.
- W2883291241 hasConcept C120665830 @default.
- W2883291241 hasConcept C121332964 @default.
- W2883291241 hasConcept C132794960 @default.
- W2883291241 hasConcept C147080431 @default.
- W2883291241 hasConcept C169150495 @default.
- W2883291241 hasConcept C169573571 @default.
- W2883291241 hasConcept C192562407 @default.
- W2883291241 hasConcept C205309187 @default.
- W2883291241 hasConcept C32891209 @default.
- W2883291241 hasConcept C40003534 @default.
- W2883291241 hasConcept C49040817 @default.
- W2883291241 hasConcept C520434653 @default.
- W2883291241 hasConcept C62520636 @default.
- W2883291241 hasConcept C67649825 @default.
- W2883291241 hasConceptScore W2883291241C102755159 @default.
- W2883291241 hasConceptScore W2883291241C110806042 @default.
- W2883291241 hasConceptScore W2883291241C120665830 @default.
- W2883291241 hasConceptScore W2883291241C121332964 @default.
- W2883291241 hasConceptScore W2883291241C132794960 @default.
- W2883291241 hasConceptScore W2883291241C147080431 @default.