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• W2883882254 abstract "Metal–organic frameworks hold a great potential for selective CO2 capture to mitigate massive CO2 emission. In this work, we report a nickel-based metal–organic framework, Ni-4PyC, with narrow and uniform ultramicropores of 6.8 A, exhibiting the CO2 adsorption capacity of 3.11 mmol/g at 298 K and 100 kPa and high CO2/N2 (0.15:0.85) and CO2/CH4 (0.5:0.5) selectivities of 51 and 6, respectively. Meanwhile, its dynamic separation performance is also confirmed by breakthrough experiments of the CO2/N2 and CO2/CH4 mixtures, further demonstrating that Ni-4PyC can selectively capture CO2 from flue gas and remove CO2 from natural gas. Molecular simulation reveals that CO2 molecules are close to the organic ligand of Ni-4PyC (pyridine), leading to CO2 being caught in the middle by two pyridines like a plier via hydrogen bonds. Besides, Ni-4PyC has an excellent recyclability without noticeable loss in CO2 adsorption after five consecutive cycles of static and dynamic adsorption experiments. These combinational meri..." @default.
• W2883882254 created "2018-08-03" @default.
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• W2883882254 date "2018-07-25" @default.
• W2883882254 modified "2023-10-16" @default.
• W2883882254 title "An Ultramicroporous Nickel-Based Metal–Organic Framework for Adsorption Separation of CO₂ over N₂ or CH₄" @default.
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• W2883882254 doi "https://doi.org/10.1021/acs.energyfuels.8b02287" @default.
• W2883882254 hasPublicationYear "2018" @default.
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