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• W2884485207 abstract "We report the results of magnetization and specific heat measurements, a 57Fe Mössbauer study of hyperfine interactions and density functional theory calculations in TlFe(MoO4)2 demonstrating two magnetic phase transitions at TN2 = 5.7 K and TN1 = 6.2 K. In the asymptotical critical region TN2 ≤ T ≤ TN1, the temperature dependence of the average hyperfine magnetic field ⟨Bhf(T)⟩ at the 57Fe nuclei is well-described by the power law ⟨Bhf(T)⟩ ∝ tβ with the static critical exponent β ≈ 0.37 inherent for a three-dimensional magnet. In this range, the Mössbauer spectra are described in terms of collinear spin-density-wave with the inclusion of high-order harmonics. The spectra of the low-temperature phase, below TN2, are well-fitted by a single six-line Zeeman pattern reflecting the equivalence of magnetic sites occupied by Fe3+ ions in an antiferromagnetic structure. The first-principles calculations allowed estimation of the strength of main exchange interactions." @default.
• W2884485207 created "2018-08-03" @default.
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• W2884485207 date "2018-07-17" @default.
• W2884485207 modified "2023-10-11" @default.
• W2884485207 title "Thermodynamic Properties, Mössbauer Study, and First-Principles Calculations of TlFe(MoO₄)₂" @default.
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• W2884485207 doi "https://doi.org/10.1021/acs.jpcc.8b05122" @default.
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