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• W2884660067 abstract "An expeditious approach to catalytic enantioselective total syntheses of crinine-type Amaryllidaceae alkaloids has been accomplished via a Pd-catalyzed enantioselective decarboxylative allylation of allylenol carbonates as a key step (up to 96% ee). Using this strategy, collective total syntheses of Amaryllidaceae alkaloids such as (−)-epi-elwesine (1b), (−)-crinine (1c), (−)-epi-crinine (1e), (−)-oxocrinine (1f), and (−)-buphanisine (1d) have been accomplished. Gratifyingly, naturally occurring Amaryllidaceae alkaloids such as (+)-vittatine (1g), (+)-epi-vittatine (1h), and (+)-epi-elwesine (1i) [enantiomers of (−)-1c, (−)-1e, and (−)-1b, respectively] have also been achieved by switching the antipode of ligand used in the catalytic enantioselective step." @default.
• W2884660067 created "2018-08-03" @default.
• W2884660067 creator A5008096601 @default.
• W2884660067 creator A5046764792 @default.
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• W2884660067 date "2018-07-20" @default.
• W2884660067 modified "2023-10-10" @default.
• W2884660067 title "Catalytic Asymmetric Total Syntheses of Naturally Occurring <i>Amarylidaceae</i> Alkaloids, (−)-Crinine, (−)-<i>epi</i>-Crinine, (−)-Oxocrinine, (+)-<i>epi</i>-Elwesine, (+)-Vittatine, and (+)-<i>epi</i>-Vittatine*" @default.
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• W2884660067 doi "https://doi.org/10.1021/acs.orglett.8b01703" @default.
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• W2884660067 hasPublicationYear "2018" @default.
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