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- W2884665034 abstract "The search for high-performance, stable, and cost-efficient membranes for vanadium flow battery (VFB) has attracted great interest. Herein, we report a physically cross-linked acid-base membrane composed of sulfonated poly(ether ether ketone) (SPEEK) and dopamine-modified halloysite nanotubes (DHNTs). The hollow structure of DHNTs allows the polymer chains getting into the lumen to form a robust mesh structure inside the composite membrane, resulting in improved mechanical stability. Meanwhile, the interface acid-base interaction between DHNTs and SPEEK facilitates the hopping of protons, leading to enhanced proton conductivity. Due to the bifunctional effects of DHNTs, the VFB with an optimized S/DHNTs 3% membrane exhibits outstanding rate performance at 40–200 mA cm−2 and excellent durability over 500 cycles at 160 mA cm−2, including extremely stable coulombic efficiency (~ 99%) and energy efficiency (~ 78%) along with very slow capacity decay rate (0.099% per cycle). The above results demonstrate that the S/DHNTs composite membrane has great advantages and broad prospects for VFB applications." @default.
- W2884665034 created "2018-08-03" @default.
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- W2884665034 date "2018-10-01" @default.
- W2884665034 modified "2023-10-16" @default.
- W2884665034 title "Bifunctional effects of halloysite nanotubes in vanadium flow battery membrane" @default.
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- W2884665034 doi "https://doi.org/10.1016/j.memsci.2018.07.033" @default.
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