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• W2885151102 abstract "The enantioselective total synthesis of an unusual pentacyclic proaporphine alkaloid, (−)-misramine, was achieved. The synthetic strategy relied on an enantioselective intramolecular Friedel–Crafts-type 1,4-addition using an asymmetric organocatalyst to construct a spiroindane skeleton containing an all-carbon quaternary stereocenter and a double reductive amination of the keto-aldehyde to form a piperidine ring toward the end of the synthesis. This work is the first example of asymmetric synthesis of a proaporphine alkaloid." @default.
• W2885151102 created "2018-08-22" @default.
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• W2885151102 date "2018-08-06" @default.
• W2885151102 modified "2023-10-18" @default.
• W2885151102 title "Enantioselective Total Synthesis of (−)-Misramine" @default.
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• W2885151102 doi "https://doi.org/10.1021/acs.orglett.8b02198" @default.
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