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- W2885151341 abstract "Ruddlesden–Popper type two-dimensional (2D) and quasi-2D perovskite-based photovoltaics have been attracting increasing attention due to their high power conversion efficiency (PCE) and long-term stability. In this work, we fabricated inverted 2D perovskite solar cells (PSCs) using a non-fullerene acceptor as electron transport material. Employing a 55-nm thick 3,9-bis(2-methylene-(3-(1,1-dicyanomethylene)-indanone))-5,5,11,11-tetrakis(5-hexylthienyl)-dithieno[2,3-d:2′,3′-d’]-s-indaceno[1,2-b:5,6-b’]dithiophene (ITIC-Th) as electron transport layer, an average PCE of 8.4% was achieved for the 2D PSCs, which was comparable to that of 2D PSCs based on phenyl-C61-butyric acid methyl ester (PCBM). However, the long-term stability of the 2D PSCs was improved as the degradation of PCE was reduced from 19.8 to 14.6% following a 15-day duration, which can be attributed to the strong hydrophobic property of the ITIC-Th. The best sample based on the 55-nm thick ITIC-Th exhibited a high PCE of 8.9% with a stable power output and negligible hysteresis, indicating the superior electron transport property of ITIC-Th. Our results demonstrate that ITIC-Th is an effective alternative to PCBM to fabricate highly efficient and stable 2D PSCs." @default.
- W2885151341 created "2018-08-22" @default.
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- W2885151341 date "2018-11-01" @default.
- W2885151341 modified "2023-10-16" @default.
- W2885151341 title "High-performance inverted two-dimensional perovskite solar cells using non-fullerene acceptor as electron transport layer" @default.
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- W2885151341 doi "https://doi.org/10.1016/j.orgel.2018.07.029" @default.
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