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• W2885152880 abstract "Highly efficient proton conductors, polyoxometalate-poly(ethylene glycol) (POM-PEG) hybrid nanocomposites, have been synthesized by encapsulating a single PEG chain inside the 1D nanochannel defined by the frameworks of POMs. By employing two types of neutron scattering techniques complemented by thermal analysis, we prove that in a nanochannel a single PEG chain stays as a distorted helix. More importantly, we reveal that the PEG segments perform a localized longitudinal random walk and quantitatively show the strong correlation between the local motion of PEG and the macroscopic proton conduction of the material. On the basis of these spatial-temporal characteristics, a microscopic picture for the proton conduction process of POM-PEG hybrid materials is proposed." @default.
• W2885152880 created "2018-08-22" @default.
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• W2885152880 date "2018-08-14" @default.
• W2885152880 modified "2023-09-30" @default.
• W2885152880 title "Spatial-Temporal Characteristics of Confined Polymer Motion Determine Proton Conduction of Polyoxometalate–Poly(ethylene glycol) Hybrid Nanocomposites" @default.
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• W2885152880 doi "https://doi.org/10.1021/acs.jpclett.8b02113" @default.
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• W2885152880 hasPublicationYear "2018" @default.
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