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- W2885281230 endingPage "12533" @default.
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- W2885281230 abstract "Inspired by the structural feature of the classical hole-transport material (HTM), Spiro-OMeTAD, many analogues based on a highly symmetrical spiro-core were reported for perovskite solar cells (PSCs). However, these HTMs were prone to crystallize because of the high molecular symmetry, forming non-uniform films, unfavorable for the device stability and large-area processing. By lowering the symmetry of spiro-core, we report herein a novel spirobisindane-based HTM, Spiro-I, which could form amorphous films with high uniformity and morphological stability. Compared to the Spiro-OMeTAD-based PSCs, those containing Spiro-I exhibit similar efficiencies for small area but higher ones for large area (1 cm2 ), and especially much higher air stability (retaining 80 % of initial PCE after 2400 h storage without encapsulation). Moreover, the Spiro-I can be synthesized from a cheap starting material bisphenol A and used with a small amount for the device fabrication." @default.
- W2885281230 created "2018-08-22" @default.
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- W2885281230 date "2018-08-23" @default.
- W2885281230 modified "2023-10-16" @default.
- W2885281230 title "Lowering Molecular Symmetry To Improve the Morphological Properties of the Hole-Transport Layer for Stable Perovskite Solar Cells" @default.
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- W2885281230 doi "https://doi.org/10.1002/anie.201807402" @default.
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