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• W2885371126 abstract "Semiconductor photocatalysis could be an effective means to combat nitrogen oxides (NO x ) based air pollution through mineralisation of NO x to nitrate. However, most of the typically TiO2-based catalysts employed show a much higher reactivity towards NO than NO2, leading to an accumulation of this unwanted and toxic intermediate. By grafting the photocatalyst with small amounts (≤0.1 at%) of isolated iron(iii) ions, the reactivity towards NO2 is increased by the factor of 9, bringing it up to par with the NO-reactivity and alleviating the problem with intermediate accumulation. Consequently, the observed selectivity of the reaction is dramatically increased from less than 40% to more than 90%. The paper also discusses possible mechanisms for this very beneficial behavior." @default.
• W2885371126 created "2018-08-22" @default.
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• W2885371126 date "2018-01-01" @default.
• W2885371126 modified "2023-09-27" @default.
• W2885371126 title "Grafted iron(<scp>iii</scp>) ions significantly enhance NO₂ oxidation rate and selectivity of TiO₂ for photocatalytic NO_x abatement" @default.
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• W2885371126 doi "https://doi.org/10.1039/c8ra05017a" @default.
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