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• W2885645087 endingPage "12577" @default.
• W2885645087 startingPage "12573" @default.
• W2885645087 abstract "Abstract Full control over multiple competing coupling sites would enable straightforward access to densely functionalized compound libraries. Historically, the site selection in Pd 0 ‐catalyzed functionalizations of poly(pseudo)halogenated arenes has been unpredictable, being dependent on the employed catalyst, the reaction conditions, and the substrate itself. Building on our previous report of C−Br‐selective functionalization in the presence of C−OTf and C−Cl bonds, we herein complete the sequence and demonstrate the first general arylations and alkylations of C−OTf bonds (in <10 min), followed by functionalization of the C−Cl site (in <25 min), at room temperature using the same air‐ and moisture‐stable Pd I dimer. This allowed the realization of the first general and triply selective sequential C−C coupling (in 2D and 3D space) of C−Br followed by C−OTf and then C−Cl bonds." @default.
• W2885645087 created "2018-08-22" @default.
• W2885645087 creator A5005884656 @default.
• W2885645087 creator A5042855471 @default.
• W2885645087 creator A5047300640 @default.
• W2885645087 date "2018-08-27" @default.
• W2885645087 modified "2023-10-17" @default.
• W2885645087 title "Modular Functionalization of Arenes in a Triply Selective Sequence: Rapid C(sp²) and C(sp³) Coupling of C−Br, C−OTf, and C−Cl Bonds Enabled by a Single Palladium(I) Dimer" @default.
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• W2885645087 doi "https://doi.org/10.1002/anie.201808386" @default.
• W2885645087 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6175235" @default.
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• W2885645087 hasPublicationYear "2018" @default.
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