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- W2885673267 abstract "Metal–organic framework (MOF)-derived porous metal/C composites have drawn considerable attention from the microwave absorption field owing to their large pore volumes and surface areas. Exploring single-MOF-derived materials with high intensity and broadband absorption is largely needed but remains a challenge. Here, porous Co/ZnO/C (CZC) microrods were fabricated easily from cuboid-shaped heterobimetallic MOFs. CZC provides an efficient platform for integrating different semiconductors (ZnO), magnetic metal (Co), and carbon sources into one particle, which enhances the electromagnetic (EM) wave-absorbing ability. The carbonization temperature which is critical for EM parameters was studied in detail. CZC annealed at 700 °C outperformed those obtained at 600 or 800 °C in terms of microwave wave-absorbing properties. The reflection loss (RL) was optimized to −52.6 (or −20.6) dB at 12.1 (or 14.8) GHz with an effective bandwidth (RL ≤ −10 dB) of 4.9 (or 5.8) GHz at the coating thickness of 3.0 (or 2.5) mm. Such enhancement of EM wave-absorbing capabilities is ascribed to the well-built porous structure, dielectric loss, and magnetic loss. This work offers a new way to prepare porous magnetic metal/C composites with excellent microwave-absorbing properties starting from heterobimetallic MOFs." @default.
- W2885673267 created "2018-08-22" @default.
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- W2885673267 date "2018-08-02" @default.
- W2885673267 modified "2023-10-16" @default.
- W2885673267 title "Highly Cuboid-Shaped Heterobimetallic Metal–Organic Frameworks Derived from Porous Co/ZnO/C Microrods with Improved Electromagnetic Wave Absorption Capabilities" @default.
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- W2885673267 doi "https://doi.org/10.1021/acsami.8b09093" @default.
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- W2885673267 hasPublicationYear "2018" @default.
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