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- W2885836998 abstract "Coupling aromatic heteronucleophiles to arenes is a common way to assemble drug-like molecules. Many methods operate via nucleophiles intercepting organometallic intermediates, via Pd-, Cu-, and Ni-catalysis, that facilitate carbon-heteroatom bond formation and a variety of protocols. We present an alternative, unified strategy where phosphonium salts can replicate the behavior of organometallic intermediates. Under a narrow set of reaction conditions, a variety of aromatic heteronucleophile classes can be coupled to pyridines and diazines that are often problematic in metal-catalyzed couplings, such as where (pseudo)halide precursors are unavailable in complex structures with multiple polar functional groups." @default.
- W2885836998 created "2018-08-22" @default.
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- W2885836998 date "2018-08-27" @default.
- W2885836998 modified "2023-10-14" @default.
- W2885836998 title "A Unified Approach to Couple Aromatic Heteronucleophiles to Azines and Pharmaceuticals" @default.
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- W2885836998 doi "https://doi.org/10.1002/anie.201807322" @default.
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