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- W2885990438 abstract "Molybdenum carbide materials are considered to be promising hydrogen evolution reaction (HER) electrocatalysts due to their similar electronic structures and catalytic activities to Pt-based catalysts. Here, we report a facile synthesis of β-Mo2C nanoparticles supported on nitrogen-doped carbon nanotubes (Mo2C/N–C) through a one-step carbonization of Mo-containing anion-doped polyaniline nanotubes. It has been revealed that the size of the obtained Mo2C nanoparticles can be effectively tuned by applying different Mo-containing anions. With MoO42– from Na2MoO4, the as-prepared Mo2C/N–C(S) with ultrasmall (2–3 nm) Mo2C nanoparticles shows excellent electrocatalytic HER activity in acidic media, with an overpotential of 189 mV vs reversible hydrogen electrode (RHE) at a geometric current density of −10 mA cm–2 and a Tafel slope of 58 mV dec–1. This study opens up a new avenue for the size-controllable synthesis of transition metal carbide nanoparticles loaded on carbon supports for energy conversion applications." @default.
- W2885990438 created "2018-08-22" @default.
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- W2885990438 date "2018-08-09" @default.
- W2885990438 modified "2023-10-17" @default.
- W2885990438 title "Anion-Induced Size Selection of β-Mo<sub>2</sub>C Supported on Nitrogen-Doped Carbon Nanotubes for Electrocatalytic Hydrogen Evolution" @default.
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- W2885990438 doi "https://doi.org/10.1021/acssuschemeng.8b02194" @default.
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