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• W2886240623 abstract "Palladium/silica (Pd/SiO2) and Pd–M/SiO2 catalysts, where M stands for sodium (Na), calcium (Ca) or barium (Ba), were studied for their catalytic ability in the partial hydrogenation of soybean oil-derived fatty acid methyl esters (SO-FAMEs) using a semibatch reactor under mild reaction conditions (4 bar hydrogen pressure and 80 °C). The catalytic performance, in terms of turnover frequency (TOF), and the selectivity toward (E)-monounsaturated FAMEs (C18:1) were investigated at 11% and 45% diunsaturated FAME (C18:2) conversion levels. The catalysts were analyzed by X-ray diffractometry, temperature-programmed desorption of carbon dioxide, transmission electron microscopy, pulse chemisorption of carbon monoxide, nitrogen adsorption–desorption, and X-ray photoelectron spectroscopy. On the one hand, the highest TOF was observed with the catalyst with the lowest basic sites on the catalyst surface (Pd–Ba/SiO2) in comparison with the other basic-modified catalysts; on the other hand, the highest selectivity toward (E)-C18:1 was evidently noticed. The oxidative stability of the partially hydrogenated SO-FAMEs (biodiesels) obtained using these catalysts could be improved 2- to 5-fold compared to those of the feed SO-FAMEs." @default.
• W2886240623 created "2018-08-22" @default.
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• W2886240623 date "2018-08-03" @default.
• W2886240623 modified "2023-09-30" @default.
• W2886240623 title "Influence of Alkaline and Alkaline Earth Metal Promoters on the Catalytic Performance of Pd–<i>M</i>/SiO₂ (<i>M</i> = Na, Ca, or Ba) Catalysts in the Partial Hydrogenation of Soybean Oil-Derived Biodiesel for Oxidative Stability Improvement" @default.
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• W2886240623 doi "https://doi.org/10.1021/acs.energyfuels.8b01498" @default.
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