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• W2886951264 abstract "Herein, we report the helical inversion of supramolecular polymeric complexes of Co 2+ containing a peptide‐based ligand comprising one alanine and three glycine moieties and an achiral terpyridine group. The helicity of the peptide‐based supramolecular polymer is controlled via strain‐induced chirality at different stoichiometric ligand/Co 2+ ratios. The supramolecular polymer S‐1 adopts octahedral geometry with right‐handed helicity (P‐type) in the presence of <0.7 equiv of Co 2+ . In contrast, it adopts coexisting octahedral and square‐pyramidal geometries in the presence of 1.0 equiv of Co 2+ and presents left‐handed helicity (M‐type). The helicities of the supramolecular polymer R‐1 with Co 2+ , prepared using the chirally opposite ligand, were completely opposite to those of S‐1 . Furthermore, the circular dichroism intensities of supramolecular polymers S‐1 and R‐1 in the presence of Co 2+ were 900–1500 times higher than those of free S‐1 and R‐1 . In addition, the helical inversion was completely reversible and controllable by the addition of more Co 2+ or ligand." @default.
• W2886951264 created "2018-08-22" @default.
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• W2886951264 date "2018-08-01" @default.
• W2886951264 modified "2023-10-06" @default.
• W2886951264 title "Helical Inversion of Peptide-based Supramolecular Co²⁺ Complexes" @default.
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• W2886951264 doi "https://doi.org/10.1002/bkcs.11540" @default.
• W2886951264 hasPublicationYear "2018" @default.
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