Matches in SemOpenAlex for { <https://semopenalex.org/work/W2887118077> ?p ?o ?g. }
- W2887118077 endingPage "2402" @default.
- W2887118077 startingPage "2393" @default.
- W2887118077 abstract "For mimicry of natural photosynthesis, particulate-based Z-scheme overall water splitting (ZOWS) free of external bias is intriguing for hydrogen production, but it commonly confronts low efficiency with the huge challenge of charge transfer and separation. Here we report an assembly of unprecedentedly efficient ZOWS system with apparent quantum efficiency (AQE) of 10.3% at 420 nm using [Fe(CN)6]3−/[Fe(CN)6]4− as redox mediator. The breakthrough of AQE is mainly ascribed to an effective cocatalyst strategy that significantly promotes charge transfer and surface catalysis. Meanwhile, the metallic Au cocatalyst is first revealed to favor electron transfer from BiVO4 to [Fe(CN)6]3− shuttle ions, and site-selective deposition of Au and CoOx dual cocatalysts on the corresponding electron-rich {010} and hole-rich {110} facets of BiVO4 is crucial for promotion of water oxidation. This work highlights the importance of the cocatalyst strategy as well as site-selective deposition in accelerating charge separation and surface catalysis of artificial photocatalyst for enhanced solar-to-chemical energy conversion." @default.
- W2887118077 created "2018-08-22" @default.
- W2887118077 creator A5010444377 @default.
- W2887118077 creator A5011065863 @default.
- W2887118077 creator A5012777183 @default.
- W2887118077 creator A5033612713 @default.
- W2887118077 creator A5054215116 @default.
- W2887118077 creator A5072555354 @default.
- W2887118077 creator A5089355761 @default.
- W2887118077 date "2018-11-01" @default.
- W2887118077 modified "2023-10-17" @default.
- W2887118077 title "Redox-Based Visible-Light-Driven Z-Scheme Overall Water Splitting with Apparent Quantum Efficiency Exceeding 10%" @default.
- W2887118077 cites W1948473998 @default.
- W2887118077 cites W1979112470 @default.
- W2887118077 cites W1979233373 @default.
- W2887118077 cites W1996929984 @default.
- W2887118077 cites W1996991937 @default.
- W2887118077 cites W2000326600 @default.
- W2887118077 cites W2001870424 @default.
- W2887118077 cites W2002140666 @default.
- W2887118077 cites W2004565790 @default.
- W2887118077 cites W2005015143 @default.
- W2887118077 cites W2008049864 @default.
- W2887118077 cites W2011187807 @default.
- W2887118077 cites W2011936672 @default.
- W2887118077 cites W2017673094 @default.
- W2887118077 cites W2025806519 @default.
- W2887118077 cites W2029198215 @default.
- W2887118077 cites W2029443292 @default.
- W2887118077 cites W2039475059 @default.
- W2887118077 cites W2040401203 @default.
- W2887118077 cites W2050525065 @default.
- W2887118077 cites W2051223431 @default.
- W2887118077 cites W2055663482 @default.
- W2887118077 cites W2063145122 @default.
- W2887118077 cites W2075307778 @default.
- W2887118077 cites W2106994275 @default.
- W2887118077 cites W2119017328 @default.
- W2887118077 cites W2131816354 @default.
- W2887118077 cites W2152931712 @default.
- W2887118077 cites W2164263712 @default.
- W2887118077 cites W2168251421 @default.
- W2887118077 cites W2257479482 @default.
- W2887118077 cites W2297655526 @default.
- W2887118077 cites W2316152954 @default.
- W2887118077 cites W2328977545 @default.
- W2887118077 cites W2338316183 @default.
- W2887118077 cites W2484985148 @default.
- W2887118077 cites W2526793459 @default.
- W2887118077 cites W2571259685 @default.
- W2887118077 cites W2606835106 @default.
- W2887118077 cites W2612652005 @default.
- W2887118077 cites W2741257603 @default.
- W2887118077 cites W2765271022 @default.
- W2887118077 cites W2776948475 @default.
- W2887118077 cites W2782830115 @default.
- W2887118077 cites W2784677805 @default.
- W2887118077 cites W2791723510 @default.
- W2887118077 doi "https://doi.org/10.1016/j.joule.2018.07.029" @default.
- W2887118077 hasPublicationYear "2018" @default.
- W2887118077 type Work @default.
- W2887118077 sameAs 2887118077 @default.
- W2887118077 citedByCount "108" @default.
- W2887118077 countsByYear W28871180772018 @default.
- W2887118077 countsByYear W28871180772019 @default.
- W2887118077 countsByYear W28871180772020 @default.
- W2887118077 countsByYear W28871180772021 @default.
- W2887118077 countsByYear W28871180772022 @default.
- W2887118077 countsByYear W28871180772023 @default.
- W2887118077 crossrefType "journal-article" @default.
- W2887118077 hasAuthorship W2887118077A5010444377 @default.
- W2887118077 hasAuthorship W2887118077A5011065863 @default.
- W2887118077 hasAuthorship W2887118077A5012777183 @default.
- W2887118077 hasAuthorship W2887118077A5033612713 @default.
- W2887118077 hasAuthorship W2887118077A5054215116 @default.
- W2887118077 hasAuthorship W2887118077A5072555354 @default.
- W2887118077 hasAuthorship W2887118077A5089355761 @default.
- W2887118077 hasBestOaLocation W28871180771 @default.
- W2887118077 hasConcept C123669783 @default.
- W2887118077 hasConcept C127413603 @default.
- W2887118077 hasConcept C159467904 @default.
- W2887118077 hasConcept C161790260 @default.
- W2887118077 hasConcept C171250308 @default.
- W2887118077 hasConcept C179104552 @default.
- W2887118077 hasConcept C185592680 @default.
- W2887118077 hasConcept C192562407 @default.
- W2887118077 hasConcept C202189072 @default.
- W2887118077 hasConcept C205507967 @default.
- W2887118077 hasConcept C35590869 @default.
- W2887118077 hasConcept C42360764 @default.
- W2887118077 hasConcept C49040817 @default.
- W2887118077 hasConcept C55493867 @default.
- W2887118077 hasConcept C55904794 @default.
- W2887118077 hasConcept C65165184 @default.
- W2887118077 hasConcept C75473681 @default.
- W2887118077 hasConcept C87803896 @default.
- W2887118077 hasConceptScore W2887118077C123669783 @default.
- W2887118077 hasConceptScore W2887118077C127413603 @default.